Impacts of Simulated Contrail Processing and Organic Content Change on the Ice Nucleation of Soot Particles
نویسندگان
چکیده
Soot particles may undergo cloud-processing during atmospheric transport after which the particle porosity and surface wettability can be modified. therefore show varying ice nucleation (IN) abilities via pore condensation freezing (PCF) mechanism, leading to poorly constrained effects on cirrus formation climate. This study simulates a typical condition (at 228 K) for size-selected (200 400 nm) aviation soot proxies with different organic contents. Based size, mass morphology changes, as well findings from parallel studies similar samples, we demonstrate that increases compactness water-interaction ability. However, availability change resulting above property changes dominates IN ability of cloud-processed PCF. Even originally organic-rich hydrophobic nucleate PCF if suitable pores generated removal cloud-processing.
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ژورنال
عنوان ژورنال: Geophysical Research Letters
سال: 2022
ISSN: ['1944-8007', '0094-8276']
DOI: https://doi.org/10.1029/2022gl099869